Annihilator of $a'$ and $b'$ in the ring $\mathbb{Z}/(a'b')$ ?

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I want to find the annihilator of $a'$ and $b'$ of the quotient ring $R=\mathbb{Z}/(a'b')$ where $a',\,b'>1$.

So if I go by the definition, $ann(a')=\{r\in\mathbb{R}\mid a'r=0\}=\{a'\mathbb{Z}+b'\mathbb{Z}+(a'\,b')\in\mathbb{R}\mid a'(a'\mathbb{Z}+b'\mathbb{Z})=0\}$

Am I correct unto this point?

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No, there are a couple of problems.

First of all, the $r\in \Bbb R$ part is not right (maybe just a typo?) It should read

$ann(a')=\{x\in\mathbb{Z}/(a'b')\mid (a'+(a'b'))x=0\}$

Secondly, it looks like you're misunderstanding the last part. If I were to rewrite the whole line, I would write this:

$$ann(a')=\{x\in\mathbb{Z}/(a'b')\mid (a'+(a'b'))x=0\}=\{z+(a'\,b')\mid (z+(a'\,b'))(a'+(a'b'))=0+(a'b')\}$$

Rewriting the expression on the far right again, we're trying to determine when $(z+(a'\,b'))(a'+(a'b'))=za'+(a'b')=0+(a'b')$. The last equality happens iff $za'\in (a'b')$.

Then $za'\in (a'b')$ implies $za'=a'b'c$ for some $c\in \Bbb Z$. Cancelling $a'$ from both sides, we arrive at $z=b'c$. Thus $z\in (b')$. So anything that annihilates $a'+(a'b')$ must lie in $(b')+(a'b')$.

Conversely, it's obvious that anything in $(b')+(a'b')$ annihilates $a'+(a'b')$.

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${\rm mod}\ ab\!:\ ax \equiv 0 \iff ab\mid ax \iff b\mid x,\ $ so $\,\ {\rm ann}(a) = (b)\,$ in $\,\Bbb Z/(ab)\ \ $ QED