Find all the numbers $a,b$ such that $\frac{2a-b}{2a+b}$ can't be reduced
Attempt:
For $a:$
$$\gcd(2a-b,2a+b)\\ =\gcd(2a-b,4a)\\ \boxed{\{a:4a\nmid2a-b\}}$$
For $b:$
$$\gcd(2a-b,2a+b)\\ =\gcd(2a-b,-2b)\\ \boxed{\{b:-2b\nmid2a-b\}}$$
I have a bad feeling about my answer
There is an error in your attempts when you write, e.g. $$ \quad \quad\gcd(2a-b,4a) \\ \to \quad \{a:4a\nmid2a-b\} $$ because it is possible that $\gcd(2a-b,4a)$ is greater than $1$, so that the fraction reduces, even while simultaneously we do not have such a strong statement as $4a$ dividing $2a - b$. (e.g. $2a-b$ is even but not divisible by $4$ or by $a$.)
Instead, here's a useful fact: $$ \gcd(xy,z) = 1 \quad\iff\quad \gcd(x,z) = 1 \text{ and } \gcd(y,z) = 1 $$ Therefore, we have that \begin{align*} \gcd(2a-b,4a) = 1 &\iff \gcd(2a-b,4) = 1 \text{ and } \gcd(2a-b,a) = 1 \\ &\iff b \text{ is odd,} \text{ and } \gcd(a,b) = 1. \\ \end{align*}
This gives you the condition you want: $a,b$ relatively prime and $b$ odd.