The projection of line $$\frac{x}{2}=\frac{y-1}{2}=\frac{z-1}{1}$$ on a plane $P$ is $$\frac{x}{1}=\frac{y-1}{1}=\frac{z-1}{-1}$$ Determine the equation of the plane.
What I tried:
Clearly, $(0,1,1)$ lies on both the plane and line.
$$\cos\theta=\dfrac{2(1)+2(1)+1(-1)}{3\sqrt3}=\dfrac1{\sqrt3}\\ \sin\theta=\sqrt{\dfrac23}$$
The angle between the line and the unit normal is $\arccos\left(\sqrt{\dfrac23}\right),$ and the unit normal is perpendicular to the projected line. Using dot product:
\begin{align} (a,b,c)\cdot(2,2,1)&=3\sqrt{\dfrac23}\\ 2a+2b+c&=\sqrt6\tag1\end{align} \begin{align} (a,b,c)\cdot(1,1,-1)&=0\\ a+b-c&=0\tag2\end{align}
But they are underdetermined. What am I doing wrong?

When setting the condition $(a,b,c)\cdot(2,2,1) = 3\sqrt{\frac{2}{3}}$ you should also set $||(a,b,c)||=1$ , otherwise it won't give you what you want and then you'll get weird results.
But $(a,b,c),(2,2,1)$ and $(1,1,-1)$ are in the same plane, so, the cross product of $(2,2,1)$ and $(1,1,-1)$ is perpendicular to $(a,b,c)$.
$$(2,2,1) \times (1,1,-1) = (-3,3,0)$$
$$(a,b,c)\cdot(-3,3,0) = 0 \iff a=b$$
Also, as you already stated, $a+b-c=0$
$a=b$ and $a+b-c=0$ , gives $c=2a$ and $b=a$. So, $N=(a,a,2a)$. In this case, it's not necessary that $||N||$ equals $1$, so $N$ may be, for example, $(1,1,2$).
So the plane you're looking for is $x + (y-1) + 2(z-1) = 0$