Let $|\vec{y}|=|\vec{x}+\vec{y}|=|\vec{x}+\vec{2y}|$. How can I find $\angle(\vec{x},\vec{y})$ without using the dot product?
How to find $\angle(\vec{x},\vec{y})$ if $|\vec{y}|=|\vec{x}+\vec{y}|=|\vec{x}+\vec{2y}|$?
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WLOG, consider $\vec{y}(1,0)$ and $\vec{x}(x_1,x_2)$. Then: $$|\vec{x}+\vec{y}|=\sqrt{(x_1+1)^2+x_2^2}=1=|y| \Rightarrow x_1^2+x_2^2+2x_1=0;\\ |\vec{x}+2\vec{y}|=\sqrt{(x_1+2)^2+x_2^2}=1=|y| \Rightarrow x_1^2+x_2^2+4x_1=-3.$$ Subtracting the two we get: $$x_1=-\frac32 \Rightarrow x_2=\pm\frac{\sqrt{3}}{2}.$$ Hence: $$\cos \theta =\frac{\vec{x}\cdot \vec{y}}{|\vec{x}|\cdot |\vec{y}|}=\frac{-\frac32+0}{\sqrt{\frac94+\frac34}\cdot 1}=-\frac{\sqrt{3}}{2} \Rightarrow \\ \theta = \frac{5\pi}{6} \ \ (\text{because the angle between vectors lies in $[0,2\pi]$}).$$ Alternatively: $$|x||y|\sin \theta=\text{abs}\begin{vmatrix}x_1&x_2 \\ y_1& y_2\end{vmatrix};\\ \sqrt{3}\cdot 1\cdot \sin \theta=\text{abs}\begin{vmatrix}-\frac32&\frac{\sqrt{3}}{2} \\ 1& 0\end{vmatrix} \Rightarrow \\ \theta = \frac{5\pi}{6} \ \ \text{(because $\vec{x}$ is in the 2nd quarter and $\vec{y}$ on the $OX^+$)};\\ \sqrt{3}\cdot 1\cdot \sin \theta=\text{abs}\begin{vmatrix}-\frac32&-\frac{\sqrt{3}}{2} \\ 1& 0\end{vmatrix} \Rightarrow \\ \theta = \frac{5\pi}{6} \ \ \text{(because $\vec{x}$ is in the 3rd quarter and $\vec{y}$ on the $OX^+$)}.$$
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A bit of geometry:
For simplicity orient $\vec y$ along the positive $x$-axis in a Cartesian coordinate system .
Add any vector $\vec x$ , i.e consider $\vec y + \vec x$.
The resulting $\vec y +\vec x$ is a vector that starts from the origin $O$ and points to the tip of $\vec y +\vec x$, and has length $|\vec y|$, i.e it lies on the Thales circle about O with radius $r:= |\vec y|$.
Let $A(0,r)$, and $B$, on the Thales circle, the tip of $\vec x + \vec y$.
$\triangle OAB$ is isosceles : $|OA|=|OB|=r.$
Let $C(-r,0)$.
Start from $C$.
The tip of $2\vec y$ is at $A$, then add $\vec x$.
Resultant is a a vector $CB$ of length $r$.
$\triangle COB$ is equilateral , side length $r$, every interior angle is $60°$,
$\triangle OAB$ is isosceles with $|OA|=|OB|=r.$
$\angle BOA =120°$,
the acute $\angle OAB =30°$,
the obtuse angle between $\vec y, \vec x$ is $150°$.

By dot product we have that
$\langle y,y\rangle=\langle x+y,x+y\rangle=\langle y,y\rangle+\langle x,x\rangle+2\langle x,y\rangle \implies \langle x,x\rangle+2\langle x,y\rangle=0$
$\langle y,y\rangle=\langle x+2y,x+2y\rangle=4\langle y,y\rangle+\langle x,x\rangle+4\langle x,y\rangle \implies 3\langle y,y\rangle=\langle x,x\rangle$
then recall
$$\cos \theta =\frac{\langle x,y\rangle}{\sqrt{\langle x,x\rangle\langle y,y\rangle}}$$
After OP editing, as an alternative by law of cosines we obtain
from which by the given conditions we obtain
$$\cos \theta =-\frac32 \frac{|y\ |}{|x|}$$
and from the triangle with sides $|x|$,$|y|$,$|x+y|$ isosceles by the condition $|y|=|x+y|$ we have
$$\frac{|x|}{2}=|y|\cos (\pi-\theta)$$
and finally, since for the above condition we need $\cos \theta <0$, we obtain
$$\cos^2 \theta=\frac 3 4\implies \cos \theta=-\frac{\sqrt 3}2$$
that is $\theta=\frac56 \pi$.