Let $M=\begin{bmatrix} a & c \\ b & d \end{bmatrix}\in SU(2)$. we have $M\overline M^t= \begin{bmatrix} aa^*+cc^* & ab^*+cd^* \\ ba^*+dc^* & bb^*+dd^* \end{bmatrix}$, and we must have $M\overline M^t=I $.
I wonder how to for these four quadratic equations to get $c=-\overline b$ and $d=\overline a$.
So far I am only able to conclude $a,d$ and $b,c $ have the same magnitudes.
Use that $$\begin{pmatrix} a & b \\ c & d \end{pmatrix}^{-1} = \frac{1}{ad-bc}\begin{pmatrix} d & -b \\ -c & a\end{pmatrix}.$$Imposing $ad-bc=1$ and setting this equal to $$\begin{pmatrix} \overline{a} & \overline{c} \\ \overline{b} & \overline{d}\end{pmatrix}$$gives the desired conclusion.