I'm preparing a talk about $\infty$-categories for a research seminar, using Luries
http://www.math.harvard.edu/~lurie/papers/croppedtopoi.pdf
as the main source. Here Lurie talks about the sets of morphisms between simplicial sets, like they are simplicial sets themselves (e.g. saying that $\hom_{Set_\Delta}(K,\mathcal{C})$ is an $\infty$-category, if $\mathcal{C}$ is an $\infty$-category.) But as far as I'm aware, he never gives an explicit description of how those sets are made into simplicial sets, and I can't find any source on this. So I want to ask, if someone knows, how this is made possible.
My approach is the following:
Define $\hom_{Set_\Delta}(S,T)_n:=\{f_n:S_n\rightarrow T_n~|~f\in\hom_{Set_\Delta}(S,T)\}$, so that the $n$-simplices are the $n$-th components of natural transformations between $S$ and $T$.
Now my problem is, how I should define the face- and degeneracy maps, since it seems impossible to me to compose in a canonical way with those maps, that come equipped with $S$ and $T$.
You can find this in Goerss-Jardine (§I.5, ``function complexes''), and here's an explanation of how to come up with the right definition.
First of all, we have finite products in $\mathbf{sSet}$: two simplicial sets $X, Y$ are presheaves $\Delta^\circ \to \mathbf{Set}$, so $X\times Y$ is defined as the product in the category of presheaves (``pointwise'': it is given by the product in $\mathbf{Set}$).
Now we would really like $\mathbf{sSet}$ to be cartesian closed: we want to define simplicial sets $\underline{\operatorname{Hom}} (Y,Z)$, in a way that $-\times Y$ is left adjoint to $\underline{\operatorname{Hom}} (Y, -)$. Note that if the adjunction holds, then the $n$-simplices of $\underline{\operatorname{Hom}} (Y,Z)$ must be given by $$\underline{\operatorname{Hom}} (Y,Z)_n \cong \operatorname{Hom}_\mathbf{sSet} (\Delta^n, \underline{\operatorname{Hom}} (Y,Z)) \cong \operatorname{Hom}_\mathbf{sSet} (\Delta^n\times Y, Z)$$ (the first isomorphism is just Yoneda).
So for every $n = 0,1,2,\ldots$ we are forced to define $$\underline{\operatorname{Hom}} (Y,Z)_n = \operatorname{Hom}_\mathbf{sSet} (\Delta^n\times Y, Z).$$ We need to make this into a simplicial set, i.e. $\underline{n} \rightsquigarrow \underline{\operatorname{Hom}} (Y,Z)_n$ should be a functor $\Delta^\circ \to \mathbf{Set}$. But this is obvious, since it is a composition of the following three functors:
A covariant functor $\Delta \to \mathbf{sSet}$ which sends $\underline{n}$ to $\Delta^n$, and a morphism $\underline{n} \to \underline{m}$ induces a morphism $\colon \Delta^n \to \Delta^m$.
A covariant functor $-\times Y\colon \mathbf{sSet}\to\mathbf{sSet}$.
A contravariant functor $\operatorname{Hom}_\mathbf{sSet} (-, Z)\colon \mathbf{sSet}^\circ \to \mathbf{sSet}$.