I would like to explain my doubt with an example.
Suppose then the Series:
$$\sum^{+\infty}_{n=1} \frac{1}{n}\tag{1}$$
I KNOW that this series is divergent. But I'm struggling on WHY this series is divergent. Actually my doubt is about why we cannot always exibit a value of the Sum of the series (or the value) and why we cannot always exibit an explicit $S_{n}$ (partial value of the infinite sequence of the sum of terms of $a_{n}$) for then apply the limit $\lim_{n\to \infty} S_{n}$.
So, in order to construct such a series we need firstly a sequence, $$\{a_{n}\}^{\infty}_{n=1} =: \Bigg\{\frac{1}{n}\Bigg\}^{\infty}_{n=1} \equiv \Bigg\{\frac{1}{1},\frac{1}{2},\frac{1}{3},...\Bigg\} \tag{2} $$
Then, with this sequence we construct another sequence:
$$ \begin{cases} S_{1} = \displaystyle \sum_{k=1}^{1} a_{k} = \frac{1}{1}\\ S_{2} = \displaystyle \sum_{k=1}^{2} a_{k} = \frac{1}{1}+\frac{1}{2}\\ S_{3} = \displaystyle \sum_{k=1}^{3} a_{k} = \frac{1}{1}+\frac{1}{2}+\frac{1}{3} \\.\\.\\.\\S_{n} = \displaystyle \sum_{k=1}^{n} a_{k} = \frac{1}{1}+\frac{1}{2}+\frac{1}{3}+...+\frac{1}{n}\\.\\.\\.\\\end{cases} $$
Called the sequence of the sum of the terms of the sequence $\Bigg\{\frac{1}{n}\Bigg\}^{\infty}_{n=1}$
$$\{S_{n}\}^{\infty}_{n=1} =: \Bigg\{ S_{1},S_{2},S_{3},...,S_{n},...\Biggr\} \equiv $$
$$ \equiv \{S_{n}\}^{\infty}_{n=1} =: \Bigg\{\Bigg(\frac{1}{1}\Bigg),\Bigg(\frac{1}{1}+\frac{1}{2}\Bigg),\Bigg(\frac{1}{1}+\frac{1}{2}+\frac{1}{3}\Bigg),...,\Bigg(\frac{1}{1}+\frac{1}{2}+\frac{1}{3}+...+\frac{1}{n}\Bigg),...\Bigg\}$$
Then we realize that "the infinite term $(S_{\infty})$ of $\{S_{n}\}^{\infty}_{n=1}$" is the "term which contains the infinite sum of the terms of the sequence $\Bigg\{\frac{1}{n}\Bigg\}^{\infty}_{n=1}$"; this is the intuition behind the object called a series:
$$S_{\infty} \equiv \sum^{+\infty}_{n=1} \frac{1}{n} = \frac{1}{1}+\frac{1}{2}+\frac{1}{3}+... \tag{3}$$
$$ * * * $$
So with the concepts presented above, we say that the series have a sum or a value if:
$$\sum^{+\infty}_{n=1} a_{n} = \lim_{n\to+\infty}S_{n}\equiv \lim_{n\to+\infty}\sum^{n}_{k=1} a_{n} = L \tag{4}$$
Well now becomes my doubt: It seems pretty clear and nature to me (even I knowing that is completely wrong) that with $(4)$ in mind we can make an procedure to find the sum for a series, which is:
$I)$ Get an sequence: $\Big\{\frac{1}{n}\Big\}^{\infty}_{n=1}$
$II)$ Write down the series: $\displaystyle \sum^{+\infty}_{n=1} \frac{1}{n}$
$III)$ Write the $S_{n}$: $\displaystyle S_{n} = \sum^{n}_{k=1} \frac{1}{k} = 1+...+\frac{1}{n}$
$IV)$ Take the limit: $ \displaystyle \lim_{n\to+\infty}\Big(1+...+\frac{1}{n}\Big)$
$V)$ Then by $(4)$ the value of $\displaystyle \sum^{+\infty}_{n=1}\frac{1}{n}$ is some number $\neq 0$
Well, this is a monstrosity. But I really need to understand why I cannot do what I did above. So, why sometimes we can "apply" the notion of $(4)$ and sometimes not?
The sum of series is the limit of $S_n$, not of $a_n$. You took the limit of $\frac{1}{n}$, while you needed to look for the limit of $S_n=1+\frac{1}{2}+...+\frac{1}{n}$. That's your mistake. Of course the sum of this series can't be $0$; this is very obvious.