Is there an intuition for the infimum definition of ${\| A \|}_{\mathrm{op}}$ without using a different, equivalent definition?
I am referring to the definition, given an operator $A: W \rightarrow V$, $$ {\| A \|}_{\mathrm{op}} = \inf \{ c \geq 0 : \| A v \| \leq c \| v \|, \ \forall v \in V \}.$$
Note that the $\sup$ definition, $$ \| A \|_{\mathrm{op}} = \sup \{ \| A v \| : v \in V, \| v \| =1 \},$$ agrees more with my intuition and I know that one can prove they are equivalent (as I have done here), but that exercise seems conceptually unrevealing.
To me the $\inf$ definition reads as choosing the smallest $c$ that bounds all vectors, however my current intuition thinks that its a better question to think about how large $A$ makes things, so rather a maximum.
I guess trivially this means things are always bounded by infinity but my point is that it doesn't really answer or correct my wrong intuition. I still feel the size of $A$ should be some sort of question about how it makes things large, so why do we consider the smallest?

The definition with the $\inf$ resembles the one used for constructing the Minkowski functional which, in turn, plays a key role in the proof of the Hahn-Banach theorem. The definition of the functional is carried out without using a norm, hence has meaning in any real vector space, normed or not. It is the use of the $\inf$ construct that allows to define the functional without the norm.
See, for example, Section 4.14 in Introductory Real Analysis, or the first chapter in Brezis's textbook on functional analysis, or Section 3.8 in Fundamentals of Functional Analysis.