I am interested in finding an upper bound for the sum $$F(n)= \sum_{l=0}^{n}\binom{n}{l}^{2}\;\sum_{j=0}^{2l-n}\binom{l}{j}$$
Ideally it should be possible to evaluate it exactly using some combinatorial identities or generating functions. Note that the $\binom{n}{l}$ term is squared, and that when $2l-n<0$, we define the inner to be zero.
Simple upper bound: By noticing that $2l-n\leq n$, we have that $$\sum_{j=0}^{2l-n}\binom{l}{j}\leq 2^n,$$ and so $$F(n)\leq 2^n \sum_{l=0}^{n}\binom{n}{l}^{2}=2^n\binom{2n}{n}.$$ (See this question for a proof that $\sum_{l=0}^{n}\binom{n}{l}^{2}=\binom{2n}{n}$) Modifying the above based on when the inner sum is zero, that is when $2l\leq n$, we can replace this upper bound by $$F(n)\leq 2^{n-1}\binom{2n}{n}.$$ However it should be possible to do significantly better than this.
By way of an intermittent progress report I submit several integral representations of the sum
$$\sum_{k=0}^n {n\choose k}^2 \times \sum_{j=0}^{2k-n} {k\choose j}.$$
They were obtained using the Egorychev method.
The reader is cordially invited to comment, verify and prove these. Saddle point asymptotics could be attempted if these were univariate integrals. I present them in the hope that perhaps a univariate generating function can be found where the catalog of asymptotics of coefficient extractor integrals could be applied. Sometimes there exist substitutions which produce radical cancellation / simplification in these binomial sum integrals.
First representation:
$$\frac{1}{2\pi i} \int_{|z|=\epsilon} \frac{(1+z)^{n}}{z^{n+1}} \frac{1}{2\pi i} \int_{|w|=\epsilon} \frac{1}{1-w} \frac{1}{w^{n+1}} (1 + w + w^2 z)^n \; dw\; dz.$$
Second representation:
$$\frac{1}{2\pi i} \int_{|z|=\epsilon} \frac{1}{z^{n+1}} (1+2z)^n (1+z)^n \; dz \\ + \frac{1}{2\pi i} \int_{|z|=\epsilon} \frac{(1+z)^{n}}{z^{n+1}} \frac{1}{2\pi i} \int_{|w|=\epsilon} \frac{1}{2w-1} \frac{1}{(1-w)^{n+1}} \frac{1}{w^n} ((1-w)^2 z + w)^n \; dw\; dz.$$
Third representation:
$$\frac{1}{2\pi i} \int_{|z|=\epsilon} \frac{1}{z^{n}} \frac{1}{2\pi i} \int_{|w|=\epsilon} \frac{1}{w^{n+1}}\frac{(1+w)^n}{1-w} \frac{1}{z-w/(1-w)} ((1+z)^2 w^2 + z)^n \; dw\; dz.$$
Fourth representation:
$$\frac{1}{2\pi i} \int_{|w|=\epsilon} \frac{1}{w^{n+1}} \frac{1}{1-w} \frac{1}{2\pi i} \int_{|z|=\epsilon} \frac{1}{z^{n+1}} (1 + z + wz)^n (1 + w^2 z)^n \; dz\; dw.$$
Fifth representation:
$$\frac{1}{2\pi i} \int_{|w|=\epsilon} \frac{1}{w^{n+1}} \frac{1}{1-w} \frac{1}{2\pi i} \int_{|z|=\epsilon} \frac{1}{z^{n+1}} \frac{1}{(1-z)^{n+1}} (1 + w - wz)^n (z + w^2 - w^2 z)^n \; dz\; dw $$
Sixth representation:
$$\frac{1}{2\pi i} \int_{|w|=\epsilon} \frac{1}{w^{n+1}} \frac{1}{1-w} \frac{1}{2\pi i} \int_{|z|=\epsilon} \frac{1}{z^{n+1}} \frac{1}{(1-z)^{n+1}} (w+1-z)^n \; dz\; dw \\ - \frac{1}{2\pi i} \int_{|w|=\epsilon} \frac{1}{w^{2n}} \frac{1}{1-w} \frac{1}{2\pi i} \int_{|z|=\epsilon} \frac{1}{z^{n+1}} \frac{1}{(1-z)^{n+1}} (w+1-z)^n (1-z + w^2 z)^n \; dz\; dw .$$