Let $\Gamma$ be a congruence subgroup of $\operatorname{SL}_2(\mathbb Z)$. The quotient $\Gamma \backslash \mathbb H$ has the structure of a one dimensional complex manifold, such that the quotient map $\pi: \mathbb H \rightarrow \Gamma \backslash \mathbb H$ is holomorphic. There is a nice fundamental domain $D \subset \mathbb H$ coming from the usual fundamental domain for $\operatorname{SL}_2(\mathbb Z)$ which, up to some boundary identification, gives us a copy of $\Gamma \backslash \mathbb H$ inside $\mathbb H$.
The Borel measure $\mu = \frac{dx dy}{y^2}$ on $\mathbb H$ descends to a Borel measure $\overline{\mu}$ on $\Gamma \backslash \mathbb H$ which we may define using the fundamental domain: if $U \subset \Gamma \backslash \mathbb H$ is Borel, then we set
$$\overline{\mu}(U) := \mu \bigg(\pi^{-1}(U) \cap D \bigg) \tag{1}$$
Now, assume $\Gamma$ is an arbitrary discrete subgroup of $\operatorname{SL}_2(\mathbb R)$.
Is there a canonical measure $\bar{\mu}$ on $\Gamma \backslash \mathbb H$ coming from $\mu = \frac{dx dy}{y^2}$?
Does there always exist a fundamental domain $D$ for $\Gamma$?
Can $\overline{\mu}$ arise from a differential form on $\Gamma \backslash \mathbb H$? That is, does $\overline{\mu}$ come from a (unique?) smooth differential $2$-form $\overline{\omega}$ on $\Gamma \backslash \mathbb H$ (thought of as a smooth manifold) which pulls back to the differential form on the smooth manifold $\mathbb H$ corresponding to $\mu = \frac{dx dy}{y^2}$?
For intuition, I'm thinking of $\mathbb R$ modulo the action of $\mathbb Z$. Up to boundary identification, $[0,1]$ is a fundamental domain for the action of $\mathbb Z$ on $\mathbb R$. For the Haar measure $\bar{\mu}$ on $\mathbb R/\mathbb Z$, we can get it in two ways. First, if $\pi: \mathbb R \rightarrow \mathbb Z$ is the quotient map, we can measure subsets of $\mathbb R/\mathbb Z$ by pulling them back to $\mathbb R$, intersecting them with $[0,1]$, then measuring. Second, $\bar{\mu}$ comes from the unique invariant nonvanishing $1$-form on $\mathbb R/\mathbb Z$ which pulls back to the top form $dx$ on $\mathbb R$ giving the Lebesgue measure on $\mathbb R$.
I'd recommend not thinking that choice of a "nice fundamental domain" is of much importance for the basic development of things. Yes, the details of a fundamental domain tell something about generators of the discrete group $\Gamma$, but that's not universally necessary, nor intelligible.
So, for example, the key relationship between functions on $\mathfrak H$ and $\Gamma\backslash \mathfrak H$, or, equivalently, $\Gamma\backslash G$ and $G$, or $\Gamma\backslash G/K$, where $G=SL_2(\mathbb R)$ and $K=SO(2,\mathbb R)$, can be described very well without any mention or choice of "fundamental domain". This is fortunate. Namely, one proves the lemma that the averaging map $f\to \sum_{\gamma\in \Gamma} f\circ \gamma$ from $C^o_c(G)$ to $C^o_c(\Gamma\backslash G)$ is surjective. Then the uniqueness of invariant distributions... shows that there is a unique integral/measure on $\Gamma\backslash G$ such that "unwinding" is correct, namely, that $$ \int_G f(g)\;dg \;=\; \int_{\Gamma\backslash G} \sum_{\gamma\in\Gamma} f(\gamma g)\;d\dot{g} $$ with $d\dot{g}$ denoting that measure on the quotient.
(Happily for us, the only things that this set-up depends upon are that $G$ be a unimodular topological group, and $\Gamma$ a discrete subgroup.)