I would like to find the integral elements int the quaternion algebra $D_{2,3}(\mathbb{Q})$. These are $2 \times 2$ matrices with elements in $\mathbb{Z}[\sqrt{2}]$ with determinant $1$. Observe these matrices are closed under multiplication.
$$ \det \left| \begin{array}{cc} x_1 + \sqrt{2} x_2 & x_3 + \sqrt{2} x_4 \\ 3(x_3 - \sqrt{2} x_4) & x_1 - \sqrt{2} x_2\end{array} \right| = x_1^2 - 2x_2^2 - 3x_3^2 + 6 x_4^2 = 1 $$ Books as recent as 2003, such on John Conway's On Quaternions and Octonions they collect fact about integral quaternions.
The usual mistake here is that I could have written an equation with no solutions, though I suspect that's unlikely. This is similar to Pell's equation and we're looking for integer points on a conic section, a hyperboloid.
By exhaustive search (a standard problem-solving heuristic) I was able to show that:
$$ \det \left| \begin{array}{cc} 4 + 3 \sqrt{2} & 7 + 5 \sqrt{2} \\ 3(7-5\sqrt{2}) & 4 - 3 \sqrt{2} \end{array}\right| = 4^2 - 2 \times 3^2 - 3 \times 7^2 + 6 \times 5^2 = 1$$ These number theory problems are notorious for their brevity. In fact, they will get arbitrarily complex. We also get an element of $D_{2,3}(\mathbb{Z})$.
There are books or papers on integer solutions to quadratic forms. Cassels' book proves outlines and theory of qudratic forms over $\mathbb{Q}$. For example, there's no complete list and even writing down generators of this group could be complicated.
You are looking for units of the order $\Lambda$ formed by the matrices, denote them $M(x_1,x_2,x_3,x_4)$ with $x_i,i=1,2,3,4,$ ranging over $\Bbb{Z}$. Obviously Conway can say more about this than I can dream of ever learning. I just wanted to make a comment explaining, why I think this is difficult. But that comment is way too long, so an answer it is.
I once had a need to find the units of a maximal order of another division algebra, but a simple computer search proved that the structure of the group is more complicated than in the case of maximal orders of number fields, and I gave up on the idea. A colleague searched for more information. A number of general facts are known, but IIRC in general the answer is rather messy. Furthermore, I have not checked whether $\Lambda$ is a maximal order of $D$. That may not be relevant you (and may not have too much of an impact on the answer), so let's ignore that question.
The main comment I want to make is that there are copies of orders of infinitely many quadratic number fields $K, [K:\Bbb{Q}]=2$ inside $\Lambda$. Consider the following. Any matrix $A=M(x_1,x_2,x_3,x_4)$ satisfies its characteristic polynomial $\chi_A(T)$. The coefficients of that polynomial are the reduced trace and norm of the element $A$ respectively. Because we are in an order we can conclude that $\chi_A(T)\in\Bbb{Z}[T]$. Furthermore, unless $A$ is in the center (= $\Bbb{Q}$), $\chi_A(T)$ cannot have rational roots. For if $\chi_A(q)=0$, $q\in\Bbb{Q}$, then $qI_2-A$ would be non-invertible contradicting the fact we have a division algebra.
It follows that the set $$ \Bbb{Q}(A)=\{q_1+q_2A\mid q_1,q_2\in \Bbb{Q}\} $$ is a splitting field of $\chi_A(T)$, call it $K_A$. That is, it is isomorphic to a quadratic number field. Furthermore, the set $$\Bbb{Z}[A]=\{n_1+n_2A\mid n_1,n_2\in\Bbb{Z}\}$$ is an order of $K_A$.
By basic facts about quadratic number fields we know that whenever $K_A$ is real (or, equivalently, the discriminant of $\chi_A(T)$ is positive), the order $\Bbb{Z}[A]$ has infinitely many units.
A few examples: $$ A=M(0,1,1,1)=\left( \begin{array}{cc} \sqrt{2} & 1+\sqrt{2} \\ 3-3 \sqrt{2} & -\sqrt{2} \\ \end{array} \right)$$ has $\chi_A(T)=T^2+1$, implying that $A$ is itself a unit of order four and $K_A\simeq \Bbb{Q}(i)$. Observe that $$ -2\cdot1^2-3\cdot1^2+6\cdot1^2=1. $$
If, instead, we look at the element $$ A=M(1,1,2,0)=\left( \begin{array}{cc} 1+\sqrt{2} & 2 \\ 6 & 1-\sqrt{2} \\ \end{array} \right) $$ we get $\chi_A(T)=T^2-2T-13$. The zeros of that polynomial are $1\pm\sqrt{14}$ implying that $\Bbb{Z}[A]\simeq \Bbb{Z}[\sqrt{14}]$. In that ring $15+4\sqrt{14}$ is a unit (solve a Pell equation to find it). The isomorphism has $A=1+\sqrt{14}$, so $$ 15+4\sqrt{14}=11I_2+4A=M(15,4,8,0) $$ should also be a unit. Indeed, $$ 15^2-2\cdot 4^2-3\cdot8^2=1. $$
Further facts/observations/complications: