In my other question here:
$$\lim_{x \rightarrow 9} \sqrt{x} = 3$$
We wanted to pick $\delta$ to satisfy $|\sqrt{x} - 3| < \epsilon$ where $0 < |x - 9| < \delta$
We can manipulate the delta equation to get $0 < |\sqrt{x} - 3| < \frac{\delta }{\sqrt{x} + 3} \leq \frac{\delta}{3}$ so we say $\delta = 3\epsilon$ is a valid choice of delta.
However, what about this instead:
$|\sqrt{x} - 3| < \epsilon$
$3-\epsilon < \sqrt{x} < 3 + \epsilon$
$(3-\epsilon)^2 < x < (3 + \epsilon)^2$
$(3-\epsilon)^2 - 9 < x - 9 < (3 + \epsilon)^2 - 9$
$|x - 9| < \min(9 - (3-\epsilon)^2 , (3 + \epsilon)^2 - 9)$
$|x - 9| < 9 - (3-\epsilon)^2$
$|x - 9| < 6 \epsilon -\epsilon^2$
Does this suggest that $\delta = 6 \epsilon -\epsilon^2$ is also a valid choice of delta? Is this the largest/widest delta bound I can use to satisfy the epsilon constraint?
This is basically correct, though to get an actual proof you would need to flesh out the logical relationships between all your inequalities to show that $|x-9|<6\epsilon-\epsilon^2$ really does imply $|\sqrt{x}-3|<\epsilon$. Note though that to prove the limit you need $\delta>0$, so this only works as a value of $\delta$ if $\epsilon<6$.
As long as $\epsilon\leq 3$, this is indeed the largest $\delta$ you can use. You can't use any larger $\delta$, since if you did, then $x=(3-\epsilon)^2$ would satisfy $0<|x-9|<\delta$ but $|\sqrt{x}-3|=\epsilon\not<\epsilon$. (The assumption that $\epsilon\leq 3$ is needed here so that $\sqrt{x}=3-\epsilon$ rather than $\epsilon-3$. If $\epsilon>3$, then it is actually impossible to have $\sqrt{x}\leq3-\epsilon$, and so the best possible $\delta$ will be $\delta=(3+\epsilon)^2-9=6\epsilon+\epsilon^2$.)