Suppose you have a triangulated region in the plane, the triangulation consisting of $n$ triangles. Take an arbitrary triangle of this triangulation and call it $\Delta_i$ with $1\leq i\leq n$.
The neighbourhood of $\Delta_i$, i.e. all the triangles around $\Delta_i$ which share a vertex or an edge with $\Delta_i$, we call this neighbourhood $N_i$.
If we can prove that you can label the vertices of $\Delta_i$ and its neighbourhood $N_i$ with just 4 colours, i.e. such that all adjacent vertices have different colour: does the 4-Colour-Theorem follow?
My thinking is: yes it follows, because $\Delta_i$ was arbitrarily chosen in this triangulation. Therefore we can conclude the whole triangulation can be 4-coloured. And if 4 colours suffice for an arbitrary triangulation, then 4 colours also suffice for any plane graph.
Would this be a valid proof strategy for the 4-Colour-Theorem, or am I taking the wrong conclusion?

If your proof strategy worked, it would prove too much.
Define a locally planar graph on a surface such as the torus to be a graph which looks like a planar graph within any "small region". (By "small", we can mean the neighborhood of a triangle, or more generally the subgraph within some fixed constant distance of any vertex). Then if your proof strategy worked, it would show that all locally planar graphs are 4-colorable as well.
However, there are counterexamples on other surfaces: for example, here is a counterexample on the torus, taken from Locally planar toroidal graphs are 5-colorable by Albertson and Stromquist. (Opposite sides of the rectangle in this diagram wrap around.)
It can be shown that in any 4-coloring of any triangulation on any surface, if there are only two vertices of odd degree, they must have the same color. However, in the example above, there are two such vertices, and they are adjacent: so this graph has no 4-coloring.
Nevertheless, we can pick any triangle within this graph, and 4-color that triangle and its neighborhood (by the 4-color theorem). It is the global properties of this graph that ultimately stop us. To take your argument, and turn it into a proof of the 4-color theorem, you would have to show that in a planar graph, there cannot be a global obstacle.