What is the value of $$ \sum_{k=0}^{n-1}\binom {n-k-1}{j-1} \binom {r+k}{j+k}$$ where $r \ge j \ge 1$?
I know that
$$ \sum_{k=0}^{n}\binom {n-k}{m}\binom{r+k}{s} = \binom {n+r+1}{m+s+1} \text{ where }n,m \ge0,\text{ and }s\ge r\ge 0$$
Please notice that second term of the first summation can be replaced by
$$ \binom {r+k}{r-j} $$
Then the first summation becomes
$$ \sum_{k=0}^{n-1}\binom {n-k-1}{j-1} \binom {r+k}{r-j} $$ which is identical to the second summation but doesn't satisfy the condition in second summation that is $ r \ngeq r - j$ since both $ r,j \ge 1 $
Is it possible to reduce the first summation similar to the second summation?
Here is some additional information which shows the two binomial expressions have different type. We transform both identities so that the different type becomes somewhat more evident. We start with a look at the second binomial identity.
We finally obtain \begin{align*} \sum_{k=t}^{n-m}\binom{n-k}{m}\binom{r+k}{r\color{blue}{+t}}=\binom{n+r+1}{m+r+t+1}\qquad\qquad n,m,r,t\geq 0\tag{1} \end{align*} Note, the lower limit of the sum starts with $k=t$, since otherwise $r+k<r+t$ and $\binom{r+k}{r+t}=0$.
We obtain
\begin{align*} \sum_{k=0}^{n-m}\binom {n-k}{m} \binom {r+k}{r\color{blue}{-(m+1)}}\qquad\qquad n,m,r\geq 0\tag{2} \end{align*}
Conclusion:
While the range of $n,m$ and $r$ is equal in both expressions (1) and (2) the range of $t\geq 0$ in (1) corresponds to the range $-(m+1)<0$.
The non-negativity of $t$ and the negativity of $-(m+1)$ is a conflict, which can't be corrected. So, the binomial expressions are of different type.
The binomial expression in (1) has $n-m-t+1$ summands, while the expression in (2) has $n-m+1$ summands.