There are two proofs of Nielsen-Schreier that I know of. The theorem states that every subgroup of a free group is free. The first proof uses topology and covering space theory and is rather elegant. The second uses combinatorial techniques on a free group of words with no relations.
Is there a more algebraic proof which somehow just uses the universal property of free groups and maybe other properties of groups that are proved more "algebraically"?
I'm interested because groups are defined purely algebraically by equations, and some proofs that a subgroup of a free abelian group is free abelian have a far more algebraic flavour. So perhaps there is some proof of Nielsen-Schreier that also has a more algebraic flavour?
Ideally I would like a proof that does not involve combinatorial properties of a group of words on generators; in other words preferably no facts from combinatorial group theory.
So the question can be marked off as answered...
I don't think there can be a "purely functorial" proof that a subgroup of a free group is free (that is, a proof using just the universal property of the free group). If there were such a proof, one would naturally expect that it can be applied to work for the relatively free groups in any variety of groups. But the only varieties of groups in which subgroups of free groups are always free are the variety of all groups, the variety of all abelian groups, and the varieties of abelian groups of prime exponent. So this argues strongly against the existence of such a proof.
As long as I'm writing this as an answer, I'll note that the technical name for such varieties is Schreier varieties. That is, a variety $\mathfrak{V}$ of algebras (in the sense of universal algebra) is said to be a Schreier variety if and only if every subalgebra of a free $\mathfrak{V}$-algebra is itself a free $\mathfrak{V}$-algebra. The proof that the only Schreier varieties of groups are the ones listed above is due to Peter Neumann and James Wiegold in Schreier varieties of groups, Math. Z. 85 (1964) 392-400. An alternate proof was given by Peter Neumann and Mike Newman, On Schreier varieties of groups, Math. Z. 98 (1967) 196-199.
A proof can also be found in Hanna Neumann's book Varieties of Groups, in section 4.3.