Is the category $\text{LCA}_c$ of connected locally compact Hausdorff abelian groups an abelian category? My feeling says no, however I can't immediately find a counterexample.
Alternatively, I'd also be happy to know whether an injective continuous map in $\text{LCA}_c$ is automatically closed.
Given an irrational number $r\in\mathbb R$, the image of the continuous injective function $\mathbb R\to\mathbb R^2/\mathbb Z^2$ given by $t\mapsto(t,rt)$ is dense but not surjective.
A reference for how to modify homological algebra so that it applies to locally compact Hausdorff abelian groups is Norbert Hoffmann and Markus Spitzweck's paper "Homological algebra with locally compact abelian groups". A reference for the more general topic of exact structures on additive categories is Theo Buehler's article Exact Categories.