I'm stuck on finding the centroid of this shape (the shaded area):
With the sphere having a radius of $r=2$, and the cardioide being given by $r=1+\cos\phi$
I found the Area, which is $A=\frac12(2\pi r^2-\frac32 \pi)=\frac{13}{4} \pi$
Now I don't know how to proceed further. Could anyone point me in the right direction? Thank you :)

Your calculated area is slightly wrong; it should be $\frac12\left(\pi r^2-\frac32\pi\right)=\frac{5\pi}4$.
We use Green's theorem to calculate the $x$- and $y$-moments, which are the sum of line integrals over the three segments of the shape. $$M_x=-\frac12\int_a^b y^2(t)x'(t)\,dt$$ $$M_y=\frac12\int_a^b x^2(t)y'(t)\,dt$$
The three segments are
So the moments are $M_x=4,M_y=-\frac{5\pi}8$. The centroid is then given by $(M_y/A,M_x/A)$ (note the swapping of arguments): $$K=\left(-\frac12,\frac{16}{5\pi}\right)$$