$$\sum_{k=1}^{n}k^2\binom{n+k}{k}$$ I tried generating function $$f=d(xd(\frac{1}{(1-x)^{n+1}})=\frac{(n+1)((n+1)x+1)}{(1-x)^{n+3}}.... (1) $$
$$=(n+1)[(n+1)x+1]\sum_{k=0}^\infty x^k\binom{n+2+k}{k}$$ On the other hand f also equals to $$\sum_{k=1}^\infty k^2\binom{n+k}{k}x^{k-1}$$ WTS sum of the first n terms' coefficients of (1) which should be $$(n+1)[\sum_{k=0}^{n-1} \binom{n+2+k}{k}+(n+1)\sum_{k=0}^{n-2} \binom{n+2+k}{k}]$$ It takes me some time to check this equals to RHS of the conclusion. Is there any other solutions?
Disclaimer
This is an incomplete combinatorial proof so I will just post it and hopefully others can improve the solution
Objects to Count
$2n+1$ people are assigned numbers from $1$ to $2n+1$ such that larger number means the person is older. Out of these people, create an organisation consisting of $n$ ordinary members, a leader, an accountant, and a secretary. The leader must be the oldest in the organisation, the accountant and secretary can be the same person.
Left Hand Side
If number $n+k+1$ is the leader, we need to choose $n$ people from number $1$ to $n+k$ to be ordinary members. Then we choose accountant and secretary from the remaining $k$ people who are also younger than the leader. The number of possibilities are given by the following expression:
$$ k^{2}\binom{n+k}{n}= k^{2}\binom{n+k}{k} $$
To obtain number of all possible organisations, we sum the expression for all possible values of $k$, which is given by the LHS in the question
$$ \sum_{k=1}^{n}k^{2}\binom{n+k}{k} $$
Right Hand Side
The organisation consists of $n+2$ person if accountant and secretary are the same person. Choose $n+2$ person, the oldest becomes the leader, then choose one person out of the rest to be both accountant and secretary.
$$ \left(n+1\right)\binom{2n+1}{n+2} $$
The organisation consists of $n+3$ person if accountant and secretary are two different people. Choose $n+3$ person, the oldest becomes the leader, choose one person out of remaining $n+2$ to be accountant, then choose one person out of remaining $n+1$ to be secretary.
$$ \left(n+2\right)\left(n+1\right)\binom{2n+1}{n+3} $$
Total number of possible organisations is given by the sum of these:
$$ \left(n+1\right)\binom{2n+1}{n+2} + \left(n+2\right)\left(n+1\right)\binom{2n+1}{n+3} = \frac{n\left(n+1\right)^{3}}{\left(n+2\right)\left(n+3\right)} \binom{2n+1}{n+1} $$
Conclusion
Since we count the number of organisations using two ways, the two expressions we obtained must be equal:
$$ \sum_{k=1}^{n}k^{2}\binom{n+k}{k} = \frac{n\left(n+1\right)^{3}}{\left(n+2\right)\left(n+3\right)} \binom{2n+1}{n+1} $$
Remark
As you might have noticed, there is some algebraic manipulation involved in obtaining the right hand side. This is why I consider this combinatorial proof incomplete.