The question is simple: how to find an unbounded operator $T:H\to H$ where $H$ is a Hilbert space such that $\text{Sp} T = \mathbb C$? This seems a very basic thing, but I have not found an example in the literature.
In some proofs, we need to consider this case separately. This example should be quite important.
Yes, such an example can be found on page 254 of Reed & Simon's Methods of Modern Mathematical Physics I.
Let $AC[0,1]$ be the family of all absolutely continuous functions on $[0,1]$ whose derivatives are in $L^2[0,1]$. Let $T:L^2[0,1] \to L^2[0,1]$ be the densely defined operator $i \frac{d}{dx}$ whose domain is the set $$ D(T) = \{ f \in L^2[0,1] : f \in AC[0,1] \}. $$ $T$ is then a closed operator whose spectrum is the entire complex plane $\Bbb C$. Indeed, observe that $$ (\lambda I - T)e^{-i\lambda x} = 0 $$ and the function $f(x) = e^{-i\lambda x}$ belongs to $D(T)$ for each $\lambda \in \Bbb C$.