So I used the Pythagorean theorem to find the missing leg first.
$$a^2 + b^2 = c^2$$
$$a^2 + 6^2 = 10^2$$
$$a^2 + 36 = 100$$
$$100 - 36 = 64$$
$$\sqrt{64} = 8$$
Now I'm just lost from here. It was just recently that I started studying tan, cos, sin etc., so any help is appreciated.

Let $\theta$ be the angle at $A$. From the perspective of $A$, we see that the side $BC$ is the "opposite" side, and $AB$ is the hypotenuse, so the ratio that is relevant here is sine:
$$\sin \theta = \frac{\textrm{opposite}}{\textrm{hypotenuse}} = \frac{6}{10} = 0.6.$$
So $\theta = \sin^{-1} 0.6$, i.e., the inverse sine of $0.6$. Notice that we didn't actually need to calculate $AC$ for this (although your work showing that $AC=8$ is correct).