The ODE in question, given below, is straightforward to solve: $$\mathbf{\ddot r} = -\omega^2 \mathbf r$$ for $\mathbf r \in \Bbb R^2$.
However, I seek to show that the general solution may be written as, $$\mathbf r = \mathbf a \sin (\omega t + \alpha) + \mathbf b \cos (\omega t + \alpha)$$ where $\mathbf a$ and $\mathbf b$ are constant and are orthogonal to each other (and $\alpha$ is a real constant).
The most general form of a solution to the ODE would be :
$\vec{\mu}=\begin{pmatrix} x_1\sin({\omega t + \alpha_1})+x_2\cos({\omega t + \alpha_2}) \\ x_3\sin({\omega t + \alpha_3})+x_4\cos({\omega t + \alpha_4}) \end{pmatrix} $
Using :
$ \sin(\alpha \pm \beta) = \sin(\alpha)\cos(\beta) \pm \cos(\alpha)\sin(\beta)$
and :
$ \cos(\alpha \pm \beta) = \cos(\alpha)\cos(\beta) \mp \sin(\alpha)\sin(\beta)$
We manipulate this into a form with two 'oscillating' vectors :
$\vec{\mu}=\begin{pmatrix} x_1\sin({\omega t +\alpha_5+ \gamma_1})+x_2\cos({\omega t +\alpha_5+ \gamma_2}) \\ x_3\sin({\omega t +\alpha_5+ \gamma_3})+x_4\cos({\omega t +\alpha_5+ \gamma_4}) \end{pmatrix} = \begin{pmatrix} x_1\sin(\omega t +\alpha_5)\cos(\gamma_1) + x_1\cos(\omega t +\alpha_5)\sin(\gamma_1)+x_2\cos(\omega t +\alpha_5)\cos(\gamma_2) - x_2\sin(\omega t +\alpha_5)\sin(\gamma_2) \\ x_3\sin(\omega t +\alpha_5)\cos(\gamma_3) + x_3\cos(\omega t +\alpha_5)\sin(\gamma_3)+x_4\cos(\omega t +\alpha_5)\cos(\gamma_4) - x_4\sin(\omega t +\alpha_5)\sin(\gamma_4) \end{pmatrix} $
$ \implies $
$\vec{\mu}=\begin{pmatrix} x'_1\sin({\omega t + \alpha_5})+x'_2\cos({\omega t + \alpha_5}) \\ x'_3\sin({\omega t + \alpha_5})+x'_4\cos({\omega t + \alpha_5}) \end{pmatrix} =\begin{pmatrix} x'_1\\ x'_3 \end{pmatrix}\sin({\omega t + \alpha_5})+ \begin{pmatrix} x'_2 \\ x'_4 \end{pmatrix}\cos({\omega t + \alpha_5}) $
With :
$x'_1:=x_1\cos(\gamma_1)-x_2\sin(\gamma_2) =x_1\cos(\alpha_1-\alpha_5)-x_2\sin(\alpha_2-\alpha_5)$
$x'_2:=x_1\sin(\gamma_1)+x_2\cos(\gamma_2)=x_1\sin(\alpha_1-\alpha_5)+x_2\cos(\alpha_2-\alpha_5)$
$x'_3:=x_3\cos(\gamma_3)-x_4\sin(\gamma_4)=x_3\cos(\alpha_3-\alpha_5)-x_4\sin(\alpha_4-\alpha_5)$
$x'_4:=x_3\sin(\gamma_3)+x_4\cos(\gamma_4)=x_3\sin(\alpha_3-\alpha_5)+x_4\cos(\alpha_4-\alpha_5)$
The vectors $\begin{pmatrix} x'_1\\ x'_3 \end{pmatrix}$ and $\begin{pmatrix} x'_2\\ x'_4 \end{pmatrix}$ are generally not yet orthogonal.
Now we show they can be made orthogonal with the right choice of $\alpha_5$ :
What we need for the vectors to be orthogonal is : $x'_1x'_2 +x'_3x'_4=0$
Solving this equation for $\alpha_5 $ gives the desired result.
It is clear that the equation can have a solution. I guess that is enough to realize it always must have a solution. Rotating the vector or changing its size can not make the above unsolvable.
For the trigonometric identities used see here. . For the main identity used below see 'Arbitrary phase shift' : $a\sin(x)+b\sin(x+\theta)=c\sin(x+\phi)$ with $c=\sqrt{a^2+b^2+2ab\cos(\theta)}$ and $\phi=atan2(b+\sin(\theta),a+b\cos(\theta))$.
$x'_1x'_2 +x'_3x'_4=0 \implies (x_1\cos(\alpha_1-\alpha_5)-x_2\sin(\alpha_2-\alpha_5))(x_1\sin(\alpha_1-\alpha_5)+x_2\cos(\alpha_2-\alpha_5))+(x_3\cos(\alpha_3-\alpha_5)-x_4\sin(\alpha_4-\alpha_5))(x_3\sin(\alpha_3-\alpha_5)+x_4\cos(\alpha_4-\alpha_5))=0$
$(x_2\sin(\alpha_2-\alpha_5)-x_1\sin(\frac{\pi}{2}+\alpha_1-\alpha_5))(x_1\sin(\alpha_1-\alpha_5)+x_2\sin(\frac{\pi}{2}+\alpha_2-\alpha_5)) +(x_4\sin(\alpha_4-\alpha_5)-x_3\sin(\frac{\pi}{2}+\alpha_3-\alpha_5))(x_3\sin(\alpha_3-\alpha_5)+x_4\sin(\frac{\pi}{2}+\alpha_4-\alpha_5))=0$
$(x_2\sin(\alpha_2-\alpha_5)-x_1\sin(\frac{\pi}{2}+\alpha_1-\alpha_2+\alpha_2-\alpha_5))(x_1\sin(\alpha_1-\alpha_5)+x_2\sin(\frac{\pi}{2}+\alpha_2-\alpha_1+\alpha_1-\alpha_5)) +(x_4\sin(\alpha_4-\alpha_5)-x_3\sin(\frac{\pi}{2}+\alpha_3-\alpha_4+\alpha_4-\alpha_5))(x_3\sin(\alpha_3-\alpha_5)+x_4\sin(\frac{\pi}{2}+\alpha_4 -\alpha_3+\alpha_3-\alpha_5))=0$
$(x_2\sin(\alpha_2-\alpha_5)+x_1\sin(\frac{3\pi}{2}+\alpha_1-\alpha_2+\alpha_2-\alpha_5))(x_1\sin(\alpha_1-\alpha_5)+x_2\sin(\frac{\pi}{2}+\alpha_2-\alpha_1+\alpha_1-\alpha_5)) +(x_4\sin(\alpha_4-\alpha_5)+x_3\sin(\frac{3\pi}{2}+\alpha_3-\alpha_4+\alpha_4-\alpha_5))(x_3\sin(\alpha_3-\alpha_5)+x_4\sin(\frac{\pi}{2}+\alpha_4 -\alpha_3+\alpha_3-\alpha_5))=0$
We define some new constants :
$\implies r_1r_2\sin(\alpha_2-\alpha_5+\phi_1)\sin(\alpha_1-\alpha_5+\phi_2) +r_3r_4\sin(\alpha_4-\alpha_5+\phi_3)\sin(\alpha_3-\alpha_5+\phi_4)=0$
$\frac{r_1r_2}{2}\cos(\alpha_2 +\phi_1 + \alpha_1+\phi_2-2\alpha_5) +\frac{r_3r_4}{2}\cos(\alpha_4 +\phi_3 + \alpha_3+\phi_4-2\alpha_5)=\frac{r_1r_2}{2}\cos(\alpha_2 +\phi_1 - \alpha_1 -\phi_2) +\frac{r_3r_4}{2}\cos(\alpha_4 +\phi_3 - \alpha_3 -\phi_4)$
$\frac{r_1r_2}{2}\sin(-\frac{\pi}{2}+\alpha_2 +\phi_1 + \alpha_1+\phi_2-2\alpha_5) +\frac{r_3r_4}{2}\sin(-\frac{\pi}{2}+\alpha_2 +\phi_1 + \alpha_1+\phi_2-2\alpha_5 + ( -\alpha_2 -\phi_1 - \alpha_1-\phi_2 +\alpha_4 +\phi_3 + \alpha_3+\phi_4 ) )=\frac{r_1r_2}{2}\cos(\alpha_2 +\phi_1 - \alpha_1 -\phi_2) +\frac{r_3r_4}{2}\cos(\alpha_4 +\phi_3 - \alpha_3 -\phi_4)$
Two more new constants :
Finally the end result :