In other words, for any symmetric or antisymmetric matrix $A\in\mathbb{R}^{n\times n}$ that has $|A_{ij}|\leq 1$, can we conclude that \begin{align*} \|A\| \leq \|J\|, \end{align*} where $\|\cdot\|$ denotes spectral norm and $J$ represents all one matrix?
Since we already know that all one matrix $J$ has the smallest eigenvalue $\sigma_n = 0$ and all other eigenvalues $\sigma_1 = \sigma_2 = \ldots = \sigma_{n-1} = n$, it is to say whether such $A$ can have singular value greater than $n$.
This is true for any matrix. In particular, we note that $\|A\| \leq \|A\|_F$, where $\|\cdot\|_F$ denotes the Frobenius norm. From there, we have $$ \|A\| \leq \|A\|_F = \sqrt{\sum_{i,j=1}^nA_{ij}^2} \leq \sqrt{\sum_{i,j=1}^n 1} = n $$