This is an extension to question 821984:
Given $N$ balls independently distributed randomly among $m$ bins, what is the probability that at least one bin gets exactly $k$ balls? And is this probability maximized when $N = k m$?
To be more clear, for fixed $N$ and $m$, there is for each integer $k$ a probability $P_{mN}(k)$ that at least one bin gets exactly $k$ balls. Is it true for all fixed $(N,m)$ that $$ \frac{N}{m} - 1 < k_0 : \max_k P_{mN}(k) = P_{mN}(k_0) < \frac{N}{m} + 1 $$
For example, for $m=3, N=7$ we get $$ P_{37}(0) = \frac{127}{729}, P_{37}(1) = \frac{409}{729}, P_{37}(2) = \frac{462}{729}, P_{37}(3) = \frac{420}{729}, \\ P_{37}(4) = \frac{280}{729}, P_{37}(5) = \frac{84}{729}, P_{37}(6) = \frac{14}{729}, P_{37}(7) = \frac{1}{729} $$ with the maximum occuring at $k=2$ which satisfies $\frac73 - 1 < 2 < \frac73+1$.
I can produce an expression for the probability, based on the probability that at least $r$ bins will contain exactly $k$ balls: $$ P(k,m,N) = \frac{1}{m^N}\sum_{r=1}^{\lfloor N/k \rfloor}(-1)^r \left( \begin{array}{c}m\\r\end{array} \right) (m-r)^{N-rk}\prod_{s=0}^{r-1} \left( \begin{array}{c}N-2s\\k\end{array} \right) $$ (The minus signs come from the usual mantra of subtracing the double-counted overlap where two bins contain $k$ balls, then adding back the triple overlap, and so forth.)
But even after wandering around in Concrete Mathematics, I can't simplify this enough to answer the maximization question.
I'm not sure if this can be simplified.
For large values of $N,m$, an asympotic approximation is straighforward (Poissonization). Letting $\lambda = N/m$, $t = \lambda/k$:
$$P \approx 1- \left( \frac{e^{-\lambda} \lambda^k}{k!}\right)^m=\\ =1- \left( \frac{k^k}{k!}\right)^m \left( t^k e^{-t k} \right)^m $$
Regarding the last expression as a function of $t$, keeping $k,m$ fixed, we get the extremum at $t=1$, as expected ($N=k m$). At this point, the value of the probability can be further approximated by the Stirling approximation, giving:
$$ P_{max}\approx 1- \left( \frac{1}{\sqrt{2 \pi k }}\right)^m$$