We have a random variable $X$ which has a Binomial Distribution Bin(n,p) and a random variable $Y$ which has a Poisson Distribution Poisson(np).
We are interested in $$f(x):=Pr[X \geq x].$$ For this we consider $$g(x):=Pr[Y \geq x]=\sum_{i=x}^{\infty} \frac{(np)^i}{i!}e^{-np}.$$
I know that the distance between These two is at most $$|f(t)-g(t)|\leq d_{TV}(Bin(n,p), Poisson(np))<p.$$
But can I say something about whether $f(x) \geq g(x)$ for all $x$ or $f(x) \leq g(x)$ for all $x$? Or is there a boundary for which $f(x)>g(x)$ or $f(x)<g(x)$?
See this question. I don't know if we can say anything pointwise about $f(x)$ vs. $g(x)$. What we can say is: $$ \large \lim_{n \to \infty, p \to 0, np = \lambda}\textrm{Binom}(n,p,k) = \textrm{Pois}(\lambda,k) $$
As a matter of fact, here are some examples which show that the Poisson and Binomial probability mass functions can be larger or smaller than the other. $$ \begin{align} \textrm{Binom}(10, .1, 3) \approx 0.057396 &< 0.61313 \approx \textrm{Pois}(1, 3)\\ \textrm{Binom}(2, .5, 1) = 0.5 &> 0.367879 \approx \textrm{Pois}(1, 1)\\ \end{align} $$